"Love-Struck" is the 5th episode of the AstroLOLogy animated series. It is the 5th part of the Rom-Antics chapter and the 5th episode overall.
The episode opens with Gemini dressed as Cupids and hiding in a bush when Cancer walks by. One of the brothers gets the idea to use their arrows to make Cancer love him, while the other aims to do the same with Sagittarius. They fight over their bow and arrow and inadvertently shoot several arrows at their intended targets. However, the girls are unaffected and promptly slap them. Gemini laugh it off as their teeth fall out.
The fortune message has one of Gemini waltzing, only for the other to knock him to the floor with an arrow to the back of his head.
"If Gemini could agree on their aim, they'd have a real shot at love."
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- This is the first time Gemini act as Cupids. The second time they wear these costumes is in "Wingmen".
- This is the first episode to have no one debut.